AMF #21 - Innovative Designs for Liquid Hydrogen (LH?) Containment Systems: A Technical Overview

AMF #21 - Innovative Designs for Liquid Hydrogen (LH?) Containment Systems: A Technical Overview

1. INTRODUCTION

The storage of hydrogen in its liquid state necessitates the maintenance of an ultra-cryogenic environment at approximately -253°C, significantly below the boiling point of LNG. This extreme temperature requirement demands the implementation of cutting-edge insulation technologies, such as vacuum insulation and Multi-Layer Insulation (MLI), at their most advanced level. The utilization of conventional insulation materials would necessitate an excessively thick insulation layer, further exacerbating the challenges posed by hydrogen's inherently low volumetric energy density.

To address these unique challenges, cargo containment systems for hydrogen are typically designed with a dual-layer insulation structure: an inner and an outer insulation layer. The inner layer spans the temperature range from near-cryogenic (close to hydrogen's boiling point) to slightly above oxygen's boiling point, while the outer layer manages the thermal gradient from this point to ambient temperature. This ensures that the extreme cold of liquid hydrogen does not compromise the integrity of the ship’s structure or pose operational hazards.

Vacuum insulation is generally preferred for the inner insulation layer due to its superior thermal resistance, however its application in large-scale shipboard cargo containment systems presents significant structural challenges. As the size of a vacuum vessel increases, the demands on its structural integrity become increasingly severe. Consequently, there is a pressing need for alternative insulation systems for larger containment structures. Hybrid insulation techniques, such as aerogel composites combined with MLI and vacuum spaces, are being explored to enhance thermal efficiency while maintaining structural feasibility.

In response to these challenges, ongoing research and development efforts are focused on creating large-capacity liquefied hydrogen carriers with innovative cargo containment systems. These designs incorporate materials such as polyurethane foam for the inner insulation layers within dedicated inner insulation spaces. To prevent condensation on the inner shell, these spaces are typically filled with gas such as hydrogen gas, which minimizes convective heat transfer and maintains pressure stability.

The development of these novel containment systems necessitated the establishment of new safety standards. To this end, the International Maritime Organization (IMO) developed the Interim Recommendations, as outlined in resolution MSC.420(97). These recommendations were crafted to facilitate the creation of tripartite agreements for pilot ships, specifically designed for researching and demonstrating the safe long-distance overseas transport of bulk liquefied hydrogen. The Interim Recommendations initially specified requirements for cargo containment systems utilizing vacuum insulation. However, recognizing the interest for larger hydrogen storage capacities, several initiatives have been undertaken to expand these recommendations to encompass new types of cargo containment systems, ensuring that safety requirements keep pace with technological advancements in the field. Additionally, fatigue assessment models for materials exposed to ultra-cryogenic conditions are under development to enhance regulatory compliance and operational safety.

Figure 1: Concept Design from Japanese Maritime Industry (Source: CCC/8/14)

2. CONTAINMENT SYSTEM DESIGN AND CONSIDERATIONS FOR LIQUID HYDROGEN STORAGE

The design of liquid hydrogen (LH?) storage tanks for maritime applications presents a multifaceted engineering challenge. These systems must not only provide exceptional insulation performance but also demonstrate resilience against the dynamic loads imposed by vessel motions. As integral components of a ship's fuel system, these tanks must address several operational factors:

  1. Fluctuating fuel levels due to consumption patterns (fuel tanks)
  2. Sloshing phenomena at various fill states
  3. Temperature gradients resulting from internal LH? movement
  4. Continuous and reliable hydrogen supply to the propulsion system (fuel tanks)
  5. Material embrittlement due to prolonged hydrogen exposure
  6. Structural deformations under varying pressure conditions
  7. Boil-off gas (BOG) management and reliquefication strategies

To effectively and safely utilize LH? for large scale marine applications, innovative designs focusing on enhanced thermal insulation performance are being explored. These advancements aim to minimize boil-off and maintain the cryogenic state of the hydrogen more efficiently. Additionally, the development of advanced composite materials for cryogenic storage, such as carbon fiber-reinforced polymer (CFRP) structures with integrated nanotechnology-enhanced insulation layers, is under investigation.

Concurrently, research is being conducted on the feasibility of incorporating newly developed stainless-steel alloys with superior yield strength and austenite stability for LH? containment. These materials show promise in significantly reducing the overall weight of fuel tanks, a critical factor in vessel design and performance optimization. Cryogenic testing and long-term hydrogen exposure evaluations are essential to qualify these materials for marine applications.

3. NOVEL DESIGN SYSTEMS FOR LH? STORAGE

Several innovative designs have been developed to enhance the efficiency and safety of LH? storage systems for maritime applications, such as:

3.1. Optimized Support Structure

The primary heat ingress in LH? tanks is considered to occur at the interconnection points between inner and outer shells. To mitigate this, a novel support structure has been proposed using topology optimization. This method is intended to maximize structural stiffness while minimizing material usage, thereby reducing thermal conduction pathways. The design is based on G10 composite material, known for its low thermal conductivity, in conjunction with stainless steel structures. Advanced computational fluid dynamics (CFD) simulations have been examined to optimize heat flux distribution and mechanical stress points in support structures.

3.2. Specialized Baffle Design

Unlike stationary LH? storage, shipboard tanks must contend with dynamic conditions such as varying fill levels and sloshing-induced forces. To address these challenges, a specialized baffle has been considered to account for LH?'s unique properties. This baffle design is intended to minimize liquid movement across various fuel levels and ship motions, thereby reducing vaporization due to sloshing. Computational modeling and physical testing in cryogenic environments are regarded as essential for evaluating baffle efficiency.

3.3. Vapor Cooled Shield (VCS)

Given the extended operational periods of ships compared to other modes of transport, continuous hydrogen supply to the propulsion system is crucial. The VCS system is intended to address the challenge of warming vaporized hydrogen (initially at -253°C) to the ambient temperatures required by propulsion systems like PEMFCs. The VCS, installed within the vacuum insulation layer, is designed to utilize high thermal conductivity copper to transfer penetrating heat to the cold vaporized hydrogen as it flows to the propulsion system. A spiral-shaped vent pipe design is considered to increase contact area, enhancing performance. Performance evaluations using LH? have been conducted to assess the VCS's effectiveness, with discharged hydrogen temperatures reaching approximately -160°C. This system not only aims to improve insulation performance but also seeks to reduce the size and capacity requirements of vaporizers.

3.4. Advanced Material Selection

STS316LH, a novel stainless-steel alloy, has been tested for LH? storage applications. This material exhibits approximately 1.8 times higher yield strength than conventional STS316L, allowing for significant weight reduction in fuel tanks. Moreover, STS316LH demonstrates enhanced austenite stability compared to STS316L, effectively mitigating concerns related to hydrogen embrittlement in cryogenic environments. Additionally, research into alternative alloys, such as aluminum-lithium composites, is ongoing to further reduce tank weight while maintaining durability under cryogenic conditions.

4. MEMBRANE CARGO CONTAINMENT SYSTEMS FOR LIQUEFIED HYDROGEN

Research and development on membrane-type cargo containment systems for LH? is currently being pursued by several organizations. These systems are considered a promising solution for large-scale LH? carriers, drawing parallels with their successful application in the LNG industry. However, the implementation of membrane systems for LH? containment necessitates the establishment and adherence to appropriate safety requirements.

A major shipbuilding company has made significant progress in this field for its membrane-type LH? containment system with plans for a pilot ship project utilizing this containment system within the next few years. Advanced numerical simulations and cryogenic impact resistance tests are being conducted to evaluate membrane containment performance

A key distinguishing feature of LH? membrane containment systems, compared to their LNG counterparts, is the operation of the inter-barrier space in a vacuum environment. The IGC Code stipulates that primary and secondary insulation spaces of membrane cargo containment systems should be inerted with a suitable dry inert gas. However, for LH? containment systems, such inerting is not practically feasible for the inter-barrier space (primary insulation space) due to the ultra-low temperature of the cargo.


Figure 2: Membrane type LH? Cargo Containment System Design Concept (Source: IMO CCC 10/14)

Consequently, maintaining the area under vacuum instead of using dry inert gas has been proposed. This operational method is not currently addressed in either the existing IGC Code or the Interim recommendations for the carriage of liquefied hydrogen in bulk (resolution MSC.420(97)) for membrane-type cargo containment systems.

The membrane cargo containment system for LH?, as illustrated in Figure 2, comprises thin liquid and gastight layers (primary and secondary barriers) supported through insulation by the adjacent hull structure. The primary and secondary insulation spaces are predominantly filled with insulation materials. The primary insulation space is maintained under vacuum during system operation, while dry inert gas is circulated throughout the secondary insulation space.

The primary purpose of maintaining a vacuum in the primary insulation space is to prevent condensation and/or solidification of gas components due to the ultra-low temperature of LH?. Only hydrogen or helium gas can be used in this space, as gases with higher boiling points are unsuitable. However, hydrogen's flammability and helium's limited commercial availability pose challenges as well.

The secondary insulation space, experiencing relatively lower heat conduction from the hydrogen cargo, is typically filled with circulating dry inert gas during normal operation. However, in the event of significant hydrogen leakage (exceeding vacuum pump capacity) detected in the primary insulation space, the secondary space should be switched to vacuum mode. Alternatively, the space may be operated in vacuum mode from the outset.

Given the complexity of these novel designs, comprehensive evaluations considering multiple factors are essential for their successful implementation and safe operation.

5. SAFETY ASSESSMENT

Membrane containment systems employ a vacuum environment, necessitating additional safety measures compared to any traditional design, such as:

  • Structural Integrity: The primary and secondary barriers, along with insulation components, must maintain structural integrity under vacuum conditions. This requirement extends beyond the standard design loads specified in the IGC Code, Finite element analysis (FEA) simulations and real-scale testing might be conducted to ensure durability.
  • Vacuum Management: The system must be capable of generating, maintaining, and monitoring the vacuum within the insulation spaces. This process is crucial for the tank's thermal efficiency and safety.
  • Emergency Preparedness: Protocols must be established to address potential emergencies, including, cargo leakage into the inter-barrier space, loss of vacuum in the insulation spaces and unanticipated temperature fluctuations due to insulation failure

6. STRUCTURAL INTEGRITY ASSESSMENT

A comprehensive strength assessment is must for all components of the cargo containment system, including:

  • Primary barrier
  • Secondary barrier
  • Structural elements within insulation spaces

This assessment must account for:

  • Vacuum environment stresses
  • Design loads as per IGC Code, Chapter 4
  • Thermal contraction and expansion
  • Potential cryogenic embrittlement

Advanced FEA and cryogenic material testing should be employed to ensure the system's resilience under all operating conditions. Large-scale validation tests simulating real shipboard conditions may also be required to be demonstrated.

7. VACUUM CONTROL SAFETY MEASURES

7.1 Vacuum Degree Specification: The required vacuum level must be precisely determined and approved by the relevant authorities, such as Administration and Class Societies. Factors influencing this specification may include:

  • Prevention of condensation or solidification of residual gases
  • Optimal thermal insulation performance
  • Structural load considerations

7.2 Pipe Routing Through Insulation Spaces: Some recommendations have been made on this issue, proposing that liquid and gas hydrogen pipes may pass through insulation spaces, provided that:

  • The vacuum level is continuously monitored
  • Pipe materials are suitable for cryogenic service
  • Thermal expansion and contraction are accounted for in the design

7.3 Vacuum Monitoring and Maintenance: A sophisticated monitoring system should be implemented to:

  • Continuously measure vacuum levels
  • Detect potential hydrogen leakage or air intrusion
  • Activate vacuum pumps as needed to maintain optimal pressure

7.4 Atmosphere Management Protocol: To mitigate the risk of flammable mixture formation:

  • Inert the spaces with dry inert gas prior to evacuation
  • Establish a detailed procedure for atmosphere handling within insulation spaces
  • Implement a purging system for periodic removal of outgassed contaminants
  • Hydrogen gas detectors should be strategically placed along vacuum pump lines for early leak detection

8. EMERGENCY CONTROL PROTOCOLS

8.1. Primary Barrier Leakage Management

Detection Methods:

  • Pressure changes in the insulation space
  • Temperature fluctuations at the secondary barrier
  • Hydrogen detection in vacuum pump lines

Response Protocol:

  • Activate a tiered emergency alarm system
  • Vent vaporized hydrogen through vacuum pump lines
  • If necessary, transition the secondary insulation space to vacuum mode
  • Isolate the primary insulation space vacuum system

8.2. Vacuum Loss Due to External Leakage

  • Operate vacuum pumps at maximum capacity
  • Monitor and control temperature to prevent air condensation
  • Initiate fault-finding procedures to locate and repair the external defect
  • Maintain the ship in a safe operational state throughout the process

8.3. Secondary Insulation Space Vacuum Loss

  • Attempt to vent intruded air via a connected vacuum pump
  • If intrusion exceeds pump capacity: Close the vacuum pump line -> Open the inert gas line -> Circulate dry inert gas to prevent air component condensation
  • Maintain a safe ship condition while addressing the underlying issue

9. Final Thoughts

The advancement of LH? containment systems marks a significant step toward sustainable maritime solutions. As the industry explores hydrogen as a viable fuel, maintaining ultra-cryogenic conditions remains a critical challenge, necessitating continuous improvements in insulation efficiency, material durability, and structural integrity. Hybrid insulation techniques and optimized structural designs are being examined to enhance performance while minimizing risks such as sloshing and heat ingress.

Safety remains at the core of LH? adoption, requiring refinements to regulatory frameworks and the integration of advanced monitoring systems. The shift toward membrane-type containment systems introduces new operational complexities, particularly in vacuum management and leakage detection, underscoring the need for further research and real-world trials. As industry stakeholders work to align technological advancements with evolving regulations, collaboration between shipbuilders, classification societies, and hydrogen technology developers will be key to ensuring reliability and scalability.

Looking ahead, the maritime sector must focus on bridging the gap between technological advancements and regulatory alignment. Collaborative efforts between stakeholders will be essential in refining best practices for LH? containment and transportation.

While substantial progress has been made, the full-scale commercialization of large capacity LH? storage in shipping requires continued investment in research and development. Efforts to improve cost efficiency, scalability, and regulatory adaptation will determine the pace at which large capacity containment systems become a mainstream reality.



Disclaimer: This article reflects the author's personal views and does not represent ABS in any way. It is not official communication from ABS, and the information here should not be taken as professional or legal advice.

Rostom Merzouki MSc CEng CMarEng MIMarEST

Director, Head of Global Gas Solutions at American Bureau of Shipping

2 周

Quite insightful review of LH2 containment systems and their challenges. Let’s not forget that the biggest challenge for LH2 transportation by sea is mainly commercial. Basically, the percentage of energy developed to produce hydrogen, then liquefying it, then maintaining it in liquid condition contained ie adressing the fugitive leakages almost equals the energy contained in the LH2 as cargo making it very expensive compared with other forms of energy. The best yield, so far, in the hydrogen value chain, is to use it next to its production sites for local communities.

Insightful. Thank you.

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